Projects per year
Abstract
Measurements of refractory and volatile components in soils from Northern England confirm 244Pu/239Pu consistent with the global average but refractory 240Pu/239Pu significantly higher but consistent with Chernobyl fallout, i.e., 0.390 ± 0.006. Refractory formation suggests temperatures > 3000°C, consistent with atmospheric injection by nuclear-driven explosions rather than by steam or hydrogen. Volatile 240Pu/239Pu is consistent with the global average, 0.181 ± 0.002, and hence lower-temperature formation in the chemical explosions and subsequent fire. This hypothesis is supported by 239Pu fission and capture cross-section enhancement due to the S-wave resonance at ~ 0.3 eV. A further calibration with a 240Pu standard is recommended to substantiate these observations.
| Original language | English |
|---|---|
| Pages (from-to) | 9287-9299 |
| Number of pages | 13 |
| Journal | Journal of Radioanalytical and Nuclear Chemistry |
| Volume | 334 |
| Issue number | 12 |
| Early online date | 20/11/2025 |
| DOIs | |
| Publication status | Published - 1/12/2025 |
User-defined Keywords
- Accelerator mass spectrometry
- Chernobyl
- Environmental plutonium
- Refractory fallout
Projects
- 1 Finished
-
AMS-UK: A UK Accelerator Mass Spectrometry Facility for Nuclear Fission Research
Joyce, M. (Principal Investigator)
Engineering and Physical Sciences Research Council
1/11/19 → 31/03/24
Project: Research
Cite this
- APA
- Author
- BIBTEX
- Harvard
- Standard
- RIS
- Vancouver